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char = (;code = 40
char = C;code = 67
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char = );code = 41
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char = c;code = 99
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char = u;code = 117
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char = e;code = 101
char = d;code = 100
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char = F;code = 70
char = e;code = 101
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char = I;code = 73
char = I;code = 73
char = I;code = 73
char = );code = 41
char = -;code = 45
char = N;code = 78
char = i;code = 105
char = (;code = 40
char = I;code = 73
char = I;code = 73
char = );code = 41
char = ;code = 32
char = c;code = 99
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char = m;code = 109
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char = e;code = 101
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char = e;code = 101
char = s;code = 115
char = ;code = 32
char = [;code = 91
char = (;code = 40
char = b;code = 98
char = p;code = 112
char = b;code = 98
char = );code = 41
char = (;code = 40
char = 2;code = 50
char = -;code = 45
char = );code = 41
char = ;code = 32
char = =;code = 61
char = ;code = 32
char = 1;code = 49
char = ,;code = 44
char = 2;code = 50
char = -;code = 45
char = b;code = 98
char = i;code = 105
char = s;code = 115
char = (;code = 40
char = p;code = 112
char = y;code = 121
char = r;code = 114
char = i;code = 105
char = d;code = 100
char = i;code = 105
char = n;code = 110
char = e;code = 101
char = -;code = 45
char = 2;code = 50
char = -;code = 45
char = c;code = 99
char = a;code = 97
char = r;code = 114
char = b;code = 98
char = o;code = 111
char = x;code = 120
char = a;code = 97
char = m;code = 109
char = i;code = 105
char = d;code = 100
char = o;code = 111
char = );code = 41
char = b;code = 98
char = e;code = 101
char = n;code = 110
char = z;code = 122
char = e;code = 101
char = n;code = 110
char = a;code = 97
char = t;code = 116
char = e;code = 101
char = ];code = 93
char = .;code = 46
result sql = [Fe(bpb)(CN)2]- as a versatile building block for the design of novel low-dimensional heterobimetallic systems: synthesis, crystal structures, and magnetic properties of cyano-bridged Fe(III)-Ni(II) complexes [(bpb)(2-) = 1,2-bis(pyridine-2-carboxamido)benzenate].

[Fe(bpb)(CN)2]- as a versatile building block for the design of novel low-dimensional heterobimetallic systems: synthesis, crystal structures, and magnetic properties of cyano-bridged Fe(III)-Ni(II) complexes [(bpb)(2-) = 1,2-bis(pyridine-2-carboxamido)benzenate].

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char = t;code = 116
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char = ;code = 32
char = s;code = 115
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char = e;code = 101
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char = s;code = 115
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char = ;code = 32
char = f;code = 102
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char = r;code = 114
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char = r;code = 114
char = a;code = 97
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char = t;code = 116
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char = e;code = 101
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char = t;code = 116
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char = r;code = 114
char = o;code = 111
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char = h;code = 104
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char = t;code = 116
char = h;code = 104
char = e;code = 101
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char = c;code = 99
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char = a;code = 97
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char = t;code = 116
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char = a;code = 97
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char = r;code = 114
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char = m;code = 109
char = a;code = 97
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char = n;code = 110
char = e;code = 101
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char = i;code = 105
char = c;code = 99
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char = s;code = 115
char = u;code = 117
char = s;code = 115
char = c;code = 99
char = e;code = 101
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char = i;code = 105
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char = i;code = 105
char = l;code = 108
char = i;code = 105
char = t;code = 116
char = y;code = 121
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char = a;code = 97
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char = i;code = 105
char = o;code = 111
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char = o;code = 111
char = f;code = 102
char = ;code = 32
char = t;code = 116
char = h;code = 104
char = e;code = 101
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char = t;code = 116
char = r;code = 114
char = i;code = 105
char = m;code = 109
char = e;code = 101
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char = i;code = 105
char = c;code = 99
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char = c;code = 99
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char = p;code = 112
char = l;code = 108
char = e;code = 101
char = x;code = 120
char = e;code = 101
char = s;code = 115
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char = y;code = 121
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char = e;code = 101
char = l;code = 108
char = d;code = 100
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char = t;code = 116
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char = e;code = 101
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char = f;code = 102
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char = l;code = 108
char = o;code = 111
char = w;code = 119
char = i;code = 105
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char = J;code = 74
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char = N;code = 78
char = i;code = 105
char = F;code = 70
char = e;code = 101
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char = ;code = 32
char = v;code = 118
char = a;code = 97
char = l;code = 108
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char = a;code = 97
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char = t;code = 116
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char = e;code = 101
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char = s;code = 115
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char = i;code = 105
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char = x;code = 120
char = c;code = 99
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char = a;code = 97
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char = e;code = 101
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char = H;code = 72
char = a;code = 97
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char = i;code = 105
char = l;code = 108
char = t;code = 116
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char = a;code = 97
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char = ;code = 32
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char = -;code = 45
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char = (;code = 40
char = N;code = 78
char = i;code = 105
char = F;code = 70
char = e;code = 101
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char = ;code = 32
char = S;code = 83
char = (;code = 40
char = N;code = 78
char = i;code = 105
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char = ;code = 32
char = (;code = 40
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char = F;code = 70
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char = 1;code = 49
char = );code = 41
char = );code = 41
char = ;code = 32
char = +;code = 43
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char = e;code = 101
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char = 2;code = 50
char = );code = 41
char = );code = 41
char = );code = 41
char = :;code = 58
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char = J;code = 74
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char = i;code = 105
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char = e;code = 101
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char = ;code = 32
char = =;code = 61
char = ;code = 32
char = 6;code = 54
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char = ,;code = 44
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char = 7;code = 55
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char = 1;code = 49
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char = ,;code = 44
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char = );code = 41
char = ;code = 32
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char = <;code = 60
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char = T;code = 84
char = H;code = 72
char = E;code = 69
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char = U;code = 85
char = D;code = 68
char = Y;code = 89
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char = O;code = 79
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char = M;code = 77
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char = C;code = 67
char = T;code = 84
char = U;code = 85
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char = A;code = 65
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char = R;code = 82
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char = T;code = 84
char = I;code = 73
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char = ;code = 32
char = R;code = 82
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char = V;code = 86
char = E;code = 69
char = A;code = 65
char = L;code = 76
char = S;code = 83
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char = H;code = 72
char = A;code = 65
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char = T;code = 84
char = H;code = 72
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char = C;code = 67
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char = B;code = 66
char = R;code = 82
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char = G;code = 71
char = I;code = 73
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char = G;code = 71
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char = H;code = 72
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char = C;code = 67
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char = X;code = 88
char = C;code = 67
char = H;code = 72
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char = ;code = 32
char = C;code = 67
char = O;code = 79
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char = P;code = 80
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char = <;code = 60
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char = N;code = 78
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char = N;code = 78
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char = N;code = 78
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char = ;code = 32
char = -;code = 45
char = ;code = 32
char = -;code = 45
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char = O;code = 79
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char = 1;code = 49
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char = N;code = 78
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char = ;code = 32
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char = e;code = 101
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char = (;code = 40
char = 1;code = 49
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char = k;code = 107
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char = T;code = 84
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char = b;code = 98
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char = (;code = 40
char = C;code = 67
char = N;code = 78
char = );code = 41
char = 2;code = 50
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char = -;code = 45
char = ;code = 32
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char = g;code = 103
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result sql = A dicyano-containing [Fe(bpb)(CN)2]- building block has been employed for the synthesis of cyano-bridged heterometallic Ni(II)-Fe(III) complexes. The presence of steric bpb(2-) ligand around the iron ion results in the formation of low-dimensional species: five are neutral NiFe2 trimers and three are one-dimensional (1D). The structure of the 1D complexes consists of alternating [NiL]2+ and [Fe(bpb)(CN)2]- generating a cyano-bridged cationic polymeric chain and the perchlorate as the counteranion. In all complexes, the coordination geometry of the nickel ions is approximately octahedral with the cyano nitrogen atoms at the trans positions. Magnetic studies of seven complexes show the presence of ferromagnetic interaction between the metal ions through the cyano bridges. Variable temperature magnetic susceptibility investigations of the trimeric complexes yield the following J(NiFe) values (based on the spin exchange Hamiltonian H = -2J(NiFe) S(Ni) (S(Fe(1)) + S(Fe(2))): J(NiFe) = 6.40(5), 7.8(1), 8.9(2), and 6.03(4) cm(-1), respectively. THE STUDY OF THE MAGNETO-STRUCTURAL CORRELATION REVEALS THAT THE CYANIDE-BRIDGING BOND ANGLE IS RELATED TO THE STRENGTH OF MAGNETIC EXCHANGE COUPLING: the larger the Ni-N[triple bond]C bond angle, the stronger the Ni- - -Fe magnetic interaction. One 1D complex exhibits long-range antiferromagnetic ordering with T(N) = 3.5 K. Below T(N) (1.82 K), a metamagnetic behavior was observed with the critical field of approximately 6 kOe. The present research shows that the [Fe(bpb)(CN)2]- building block is a good candidate for the construction of low-dimensional magnetic materials.

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